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Organic Transistors
In article number 2210093, Yan Zhao, Yang Wang, Yunqi Liu, and co‐workers demonstrate a hybrid acceptor‐modulation strategy to synthesize an acceptor unit with a fluorinated triple‐acceptor architecture (DPP–difluorobenzothiadiazole–DPP (DFB)). The DFB‐based semiconducting polymers feature low‐lying frontier molecular orbital levels, shape‐persistent backbones, and high crystallinity,...
The development of unipolar n‐type semiconducting polymers with electron mobility (µe) over 5 cm2 V−1 s−1 remains a massive challenge in organic semiconductors. Diketopyrrolopyrrole (DPP) has proven to be a successful unit for high‐performance p‐type and ambipolar polymers. However, DPP's moderate electron‐accepting capability leads to the shallow frontier molecular orbital (FMO) levels of the resultant...
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