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The selective oxidation of lower alkanes, such as ethane, remains a major research challenge in catalysis. In this study Fe and Cu containing zeolites are investigated as catalysts for the production of C2 oxygenated products from ethane using H2O2 as an oxidant. We utilise a trickle bed reactor to effectively control the contact time between reactants and catalyst to minimise C–C scission and over...
A series of bismuth molybdate catalysts were compared using a continuous feed of isobutene in air or a cyclic/pulse or gas–gas periodic flow mode, in which the oxide is first treated with air at the reaction temperature, followed by reaction of isobutene in nitrogen or argon in the absence of oxygen. For nonpromoted catalysts, in the continuous-feed mode, relatively low selectivities for methacrolein...
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