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Light, polymer, action: A set of water‐soluble poly(acrylic acid) catalysts PAA‐g‐Fe2S2 containing {Fe2S2}, an [FeFe]‐hydrogenase active‐site mimic, is synthesized. This system, combined with CdSe quantum dots and ascorbic acid, has an exceptional turnover number and initial turnover frequency (27 135 and 3.6 s−1) for the photocatalytic production of H2 in water, which is the highest efficiency to...
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