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This work reports the dehydrated Zr‐based MOF UiO‐66(SH)2 as a visible‐light‐driven photocatalyst to mimic the biological N2 fixation process. The 15N2 and other control experiments demonstrated that the new photocatalyst is highly efficient in converting N2 to ammonia. In‐situ TGA, XPS, and EXAFS as well as first‐principles simulations were used to demonstrate the role of the thermal treatment and...
This work reports the dehydrated Zr‐based MOF UiO‐66(SH)2 as a visible‐light‐driven photocatalyst to mimic the biological N2 fixation process. The 15N2 and other control experiments demonstrated that the new photocatalyst is highly efficient in converting N2 to ammonia. In‐situ TGA, XPS, and EXAFS as well as first‐principles simulations were used to demonstrate the role of the thermal treatment and...
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