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The synthesis and single-crystal X-ray structure of an ion-pair complex, [4,4 ' -H 2 bpy][Cu(mnt) 2 ] (1), is described. In the crystal structure, the interactions between anions and cations via bifurcated (bpyN)-H...(NC-mnt) 2 hydrogen bonds give rise to a three-dimensional supramolecular network having well-defined channels. Complex 1 exhibits two redox waves at +0...
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