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Our recent studies of the steady-state kinetics of the N 2 O–CO reaction on Rh(110) indicate that at CO excess, the reaction rate increases with increasing temperature. At N 2 O excess, the reaction rate is nearly independent of temperature at T<520K and rapidly decreases with increasing temperature at T>520K. Our present analysis of the relevant data indicates that the latter...
Experimental studies indicate that the N 2 O–CO reaction occurring on Pd(110) under UHV conditions exhibits a first-order kinetic phase transition in the steady-state case and also transient kinetics strongly dependent on the initial state of the system. We construct a mean-field kinetic model describing these phenomena. With a minimal number of the fitting parameters, the model reasonably...
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