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Ruthenium (Ru) is an ideal substitute to commercial Pt/C for hydrogen evolution reaction (HER). Reducing the size of Ru to clusters can greatly increase the utilization of atoms, however, over‐strong RuH binding will be brought about. Additionally, the water dissociation ability of Ru clusters is unfavorable, leading to unsatisfactory activity in alkaline and neutral HER. Herein, a rational and versatile...
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