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The gas solubility in 1‐dodecyl‐3‐methylimidazolium [C12MIM] based ionic liquids (ILs) was measured at temperatures (333.2, 353.2, and 373.2) K and pressures up to 60 bar for the first time. The popular UNIFAC‐Lei model was successfully extended to long‐chain imidazolium‐based IL and gas (CO2, CO, and H2) systems. The free volume theory was used to explain the gas solubility and selectivity in imidazolium‐based...
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