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Stereocontrolled formation of carbon−carbon and carbon−heteroatom bonds through asymmetric organocatalysis is a formidable challenge for modern synthetic chemistry. Among the most significant contributions to this field are the transformations involving the use of acetaldehyde or α‐heteroatom‐substituted acetaldehydes for constructing valuable synthons (e.g., amino acid derivatives and hydroxycarbonyl)...
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