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When a racemic mixture of chiral building blocks self‐assembles to form discrete molecular or supramolecular cages, the system can adopt either social or narcissistic chiral self‐sorting. However, control over such chiral self‐sorting is hard to achieve with a desired choice of outcome. Herein, we report anion templated high‐fidelity chiral self‐sorting during the coordination‐driven self‐assembly...
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