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A particular challenge in the design of organic photosensitizers (PSs) with donor–acceptor (D‐A) structures is that it is based on trial and error rather than specific rules. Now these challenges are addressed by proposing two efficient strategies to enhance the photosensitization efficiency: polymerization‐facilitated photosensitization and the D‐A even–odd effect. Conjugated polymers have been found...
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