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Polar photovoltaic effect (PPE) has attracted great attention in regulating desired optoelectronic properties, which can be driven by order–disorder and displacive phase transitions. Bond‐switching is also a feasible method to induce PPE, but such investigation is very rare. Lead‐halide hybrid perovskite (LHHP) is an outstanding photodetection material; lead atoms possess rich coordination modes to...
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