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While self‐assembled molecular building blocks could lead to many next‐generation functional organic nanomaterials, control over the thin‐film morphologies to yield monolithic sub‐5 nm patterns with 3D orientational control at macroscopic length scales remains a grand challenge. A series of photoresponsive hybrid oligo(dimethylsiloxane) liquid crystals that form periodic cylindrical nanostructures...
In article number 1701043, Albertus P. H. J. Schenning and co‐workers, explore how photo‐responsive small molecules can be monolithically aligned when exposed to linearly polarized light in thin films with sub‐5 nm cylindrical nanopatterns, while when exposed to unpolarized light the self‐assembled nanocylinders are aligned out‐of‐plane. These results pave the way for generating defect‐free functional...
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