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Reactions of acrolein, water, and oxygen with the vacuum-reduced surface of TiO 2 (110) are reported in a temperature programmed reaction study of the interaction of an aldehydic pollutant with a reducible metal oxide. A total of 25% of the acrolein that binds to the surface is converted to products. Notably, carbon–carbon coupling occurs with 86% selectivity for formation of C 6 products:...
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