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All crystals are not ideal, and many of their properties are often determined not by the regular arrangement of atoms, but by the irregular arrangement of crystal defects. Many properties of materials can be controlled effectively by proper use of solid defects. By substitution of NH4+ ion of a hexagonal perovskite structure (H2dabco)(NH4)(NO3)3 (dabco=1,4‐diazabicyclo[2.2.2]octane, 1) with Cd2+ ion,...