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Cyclopentadienyl (Cp) ligands enable efficient steering of various transition‐metal‐catalyzed transformations, in particular enantioselective C−H activation. Currently only few chiral Cp ligands are available. Therefore, a conceptually general approach to chiral Cp ligand discovery would be invaluable as it would enable the discovery of applicable Cp ligands and to efficiently and rapidly vary and...
Trienamin‐Aktivierung wurde für die Entwicklung einer γ,δ‐regioselektiven Diels‐Alder‐Reaktion mit elektronenarmen β‐substituierten 2,4‐Dienen und 2,4‐Dienalen genutzt. Die resultierenden multifunktionellen Cycloaddukte enthalten perfekt positionierte funktionelle Gruppen, wodurch ein 1,5‐Hydridtransfer von der C‐H‐Gruppe eines Aldehyds an ein aktiviertes Alken unter sequenzieller Katalyse eines Carbens...
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