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Refluxing azoimine ligand containing terminal acetylene group (L=C6H5NNC(COCH3)NC6H4CCH) with RuCl3·3H2O in ethanol resulted hydrating the terminal acetylene group to the corresponding enol form C6H5NNC(COCH3)NC6H4C(OH)CH2 (L1), ketone form C6H5NNC(COCH3)NC6H4COCH3 (L2) and vinyl chloride: C6H5NNC(COCH3)NC6H4C(Cl)CH2 (L3) via Markovnikov selectivity. Ruthenium complexes of the later ligands and α-diamines...
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