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A new approach to allylic alkylation is realized using an atomically dispersed palladium catalyst (Pd1/TiO2‐EG). Unlike conventional methods that require derivation of substrates and utilization of additives, this method allows for direct allylic alkylation from allylic alcohols, producing H2O as the sole by‐product. The catalyst's high efficiency is attributed to the local hydrogen bonding at the...
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