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In article number 1801931, Jinlan Wang, Wei Chen, and co‐workers develop a new strategy to enhance the near‐infrared absorption and optoelectronic performance of 2D black phosphorus via Ag nanoclusters functionalization. It is shown that Ag–P hybridization induces localized gap states, thus activating a new optical transition route in the near‐infrared region.
Black phosphorus (BP), as a fast emerging 2D material, shows promising potential in near‐infrared (NIR) photodetection owing to its relatively small direct thickness‐dependent bandgaps. However, the poor NIR absorption due to the atomically thin nature strongly hinders the practical application. In this study, it is demonstrated that surface functionalization of Ag nanoclusters on 2D BP can induce...
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