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The LiNiO2 (LNO) positive electrode material is one of the most promising high‐voltage alternatives for the layered oxide materials such as LiCoO2 (LCO). However, the poor cyclability still limits widespread commercialization of LNO, whereas crack formation is one of the main issues leading to its premature aging. In this study, a series of Al‐doped LNO (LiNi1−xAlxO2, x = 0, 0.02, 0.04, 0.06) positive...
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