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All‐solid‐state batteries (ASSBs) represent a highly promising next‐generation energy storage technology owing to their inherently high safety, device reliability, and potential for achieving high energy density in the post‐ara of lithium‐ion batteries, and therefore extensive searches are ongoing for ideal solid‐state electrolytes (SSEs). Though promising, there is still a huge barrier that limits...
The microstructure of hard carbons (HCs) including interlayer distance and lateral ab direction and pore size distribution plays a key role in regulating the sodium ions storage performance. Herein, by employing the gelatinous agar as a model precursor, series P‐doping HCs (P‐HC‐x, x = 1, 2, 3, 4) are facilely prepared in batches via controllably regulating its crosslinking state by phytic acid (PA)...
Achieving a balance between H‐atom adsorption and binding with H2 desorption is crucial for catalyzing hydrogen evolution reaction (HER). In this study, the feasibility of designing and implementing built‐in opposite electric fields (OEF) is demonstrated to enable optimal H atom adsorption and H2 desorption using the Ni3(BO3)2/Ni5P4 heterostructure as an example. Through density functional theory...
The rapid evolution of smart grid system urges researchers on exploiting systems with properties of high‐energy, low‐cost, and eco‐friendly beyond lithium‐ion batteries. Under the circumstances, sodium‐ and potassium‐ion batteries with the semblable work mechanism to commercial lithium‐ion batteries, hold the merits of cost‐effective and earth‐abundant. As a result, it is deemed a promising candidate...
Phosphorene is a 2D phosphorus atomic layer arranged in a honeycomb lattice like graphene but with a buckled structure. Since its exfoliation from black phosphorus in 2014, phosphorene has attracted tremendous research interest both in terms of synthesis and fundamental research, as well as in potential applications. Recently, significant attention in phosphorene is motivated not only by research...
Robust, ultrathin, and environmental‐friendliness papers that synergize high‐efficiency electromagnetic interference (EMI) shielding, personal thermal management, and wearable heaters are essential for next‐generation smart wearable devices. Herein, MXene nanocomposite paper with a nacre‐like structure for EMI shielding and electrothermal/photothermal conversion is fabricated by vacuum filtration...
Near‐neutral zinc–air batteries (ZABs) have garnered significant research interest due to their high energy density, exceptional electrochemical reversibility, and adaptability to ambient air. However, these batteries suffer from substantial electrochemical polarization, low energy efficiency, and poor rate performance. In this study, a mesoporous carbon (meso‐C) with a high specific surface area...
Glioblastoma (GBM), the most aggressive and lethal form of malignant brain tumor, is a therapeutic challenge due to the drug filtration capabilities of the blood‐brain barrier (BBB). Interestingly, glioblastoma tends to resist apoptosis during chemotherapy, but is susceptible to ferroptosis. Developing therapies that can effectively target glioblastoma by crossing the BBB and evoke ferroptosis are,...
On account of high capacity and high voltage resulting from anionic redox, Li‐rich layered oxides (LLOs) have become the most promising cathode candidate for the next‐generation high‐energy‐density lithium‐ion batteries (LIBs). Unfortunately, the participation of oxygen anion in charge compensation causes lattice oxygen evolution and accompanying structural degradation, voltage decay, capacity attenuation,...
Aqueous Zinc Batteries
In article number 2301770, Yueliang Gu, Xiaochuan Ren, Daming Zhu, Jianxin Zou, and co‐workers elucidate the reaction mechanism of Mn2+ electrolyte additives in aqueous zinc batteries (ZIBs) via operando synchrotron X‐ray diffraction, ex situ X‐ray absorption spectroscopy and electrochemical analyses. A reversible Mn2+/MnO2 deposition/dissolution reaction occurred at the cathode,...
Aqueous zinc batteries (ZIBs) have attracted considerable attention in recent years because of their high safety and eco‐friendly features. Numerous studies have shown that adding Mn2+ salts to ZnSO4 electrolytes enhanced overall energy densities and extended the cycling life of Zn/MnO2 batteries. It is commonly believed that Mn2+ additives in the electrolyte inhibit the dissolution of MnO2 cathode...
Amination of aryl chlorides by metallaphotocatalysis is highly desired but remains practically challenging. Meanwhile, relying on soluble noble‐metal photocatalysts suffers from resource scarcity and structural instability which limit their practical application. Here in, a highly crystalline acetylene‐based hydrazone‐linked covalent organic framewok‐1 (AC‐COF‐1) is reported that enables metallaphotocatalytic...
The advancement in thermosensitive active hydrogels has opened promising opportunities to dynamic full‐thickness skin wound healing. However, conventional hydrogels lack breathability to avoid wound infection and cannot adapt to wounds with different shapes due to the isotropic contraction. Herein, a moisture‐adaptive fiber that rapidly absorbs wound tissue fluid and produces a large lengthwise contractile...
Although tremendous progress has recently been made in quasi‐2D perovskite light‐emitting diodes (PeLEDs), the performance of red PeLEDs emitting at ≈650–660 nm, which have wide prospects for application in photodynamic therapy, is still limited by an inefficient energy transfer process between the quasi‐2D perovskite layers. Herein, a symmetric molecule of 3,3′‐(9H‐fluorene‐9,9‐diyl)dipropanamide...
The design and synthesis of novel two‐dimensional (2D) materials that possess robust structural stability and unusual physical properties may open up enormous opportunities for device and engineering applications. Herein, a 2D sumanene lattice that can be regarded as a derivative of the conventional Kagome lattice is proposed. The tight‐binding analysis demonstrates sumanene lattice contains two sets...
Vascularized osteogenesis is essential for successful bone regeneration, yet its realization during large size bone defect healing remains challenging due to the difficulty to couple multiple biological processes. Herein, harnessing the intrinsic angiogenic potential of vascular derived extracellular matrix (vECM) and its specific affinity to growth factors, a vECM/GelMA based hybrid hydrogel delivery...
Tellurium (Te) is a promising electrode active material for potassium‐ion batteries due to its intrinsic electrical conductivity and ultra‐high theoretical volumetric capacity. Nevertheless, Te‐based electrodes usually exhibit low capacity at high rates and poor cycling stability caused by the large volume expansion and severe polytellurides dissolution. Herein, hierarchical porous carbon nanofibers...
Germanium (Ge)‐based devices are recognized as one of the most promising next‐generation technologies for extending Moore's law. However, one of the critical issues is Fermi‐level pinning (FLP) at the metal/n‐Ge interface, and the resulting large contact resistance seriously degrades their performance. The insertion of a thin layer is one main technique for FLP modulation; however, the contact resistance...
Recent years have witnessed the rapid development of sustainable materials. Along this line, developing biodegradable or recyclable soft electronics is challenging yet important due to their versatile applications in biomedical devices, soft robots, and wearables. Although some degradable bulk hydrogels are directly used as the soft electronics, the sensing performances are usually limited due to...
Two‐dimentional semiconductors have shown potential applications in multi‐bridge channel field‐effect transistors (MBC‐FETs) and complementary field‐effect transistors (C‐FETs) due to their atomic thickness, stackability, and excellent electrical properties. However, the exploration of MBC‐FET and C‐FET based on large‐scale 2D semiconductors is still lacking. Here, based on a reliable vertical stacking...
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