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Novel bis-styryl dyes based on a quaternized centrosymmetrical benzodipyrrolenine moiety were synthesized by reaction of a quaternized benzodipyrrolenine with two equivalents of 4-dimethylaminobenzaldehyde, 4-dimethylaminocinnamoic aldehyde or 4-(3,5-diphenyl-4,5-dihydro-1H-1-pyrazolyl)benzaldehyde. The molecular structures and spectral properties of these dyes were investigated using PM3 and PPP...
A novel method of synthesizing long-wavelength absorbing and emitting bis-trimethine dyes that consists of condensing benzodipyrrolenine dialdehyde with quaternized heterocyclic CH-acidic compounds was used to prepare a series of biscyanines. The new method is more convenient than its conventional counterepart, which relies upon condensation of a quaternized benzodipyrrolenine with Fisher's aldehyde,...
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