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The use of water as reaction medium in the heterogeneous activation of C–H bonds has numerous advantages in terms of environmental benign, safety and cost efficiency impact. However, it is severely hampered because the reactants are difficult to dissolve in water and contact with the active sites of heterogeneous catalysts. Herein, we choose perfluoroalkane-functionalized mesoporous metal-organic...
Metal–organic frameworks (MOFs) in most metal nanoparticles (NPs)/MOFs composite catalysis systems serve only as supports to protect NPs from agglomeration. Up to now, most MOFs have still been largely restricted to the microporous regime, which limits the diffusion and mass transfer of substrates and products. Here, we use hierarchically micro- and mesoporous MOFs for the first time to immobilize...
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