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We observe large vibrationally-induced modulations in high order harmonic conversion in N2O4. We explain this unexpected result as due to the changing electronic structure induced by the vibration, leading to preferential emission at the outer turning point of the vibration.
We observe large vibrationally-induced modulations in high order harmonic conversion in N2O4. We explain this unexpected result as due to the changing electronic structure induced by the vibration, leading to preferential emission at the outer turning point of the vibration.
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