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The carbon dioxide reduction reaction (CO2RR) driven by electricity can transform CO2 into high‐value multi‐carbon (C2+) products. Copper (Cu)‐based catalysts are efficient but suffer from low C2+ selectivity at high current densities. Here La(OH)3 in Cu catalyst is introduced to modify its electronic structure towards efficient CO2RR to C2+ products at ampere‐level current densities. The La(OH)3/Cu...
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