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Planar gliding along with anisotropic lattice strain of single‐crystalline nickel‐rich cathodes (SCNRC) at highly delithiated states will induce severe delamination cracking that seriously deteriorates LIBs’ cyclability. To address these issues, a novel lattice‐matched MgTiO3 (MTO) layer, which exhibits same lattice structure as Ni‐rich cathodes, is rationally constructed on single‐crystalline LiNi...
Intergranular cracking of Ni‐rich layered LiNi1‐x‐yCoxMnyO2 (1‐x‐y ≥ 0.8) cathode particles deteriorate the chemo–electro–mechanical stability of high‐energy lithium‐ion batteries (LIBs), thus presenting a challenge to typical modification methods to establish robust structures with highly efficient lithium‐ion storage. Herein, the ZrTiO4 (ZTO) as an epitaxial layer to enhance mechanical stability...