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The charge carrier transport of conjugated polymer thin film is mainly decided by the crystalline domain and intercrystallite connection. High‐density tie‐chain can provide an effective bridge between crystalline domains. Herein, the tie‐chain connection behavior is optimized by decreasing the crystal region length (lc) and increasing the crystallization rate. Poly[4‐(4,4‐bis(2‐octyldodecyl)‐4H‐cyclopenta[1,2‐...
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