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Ammonia (NH3) is an essential chemical for agricultural production and a promising next‐generation hydrogen‐rich fuel. The electrocatalytic nitrate (NO3−) reduction reaction (NO3RR) to NH3 provides a sustainable and low‐energy method to replace industrial NH3 synthesis. However, the NO3− to NH3 conversion is limited by the complex eight‐electron and nine‐proton reduction processes, thus it is highly...