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Fully conjugated porous aromatic frameworks (PAFs) have been constructed through Gilch reaction. The obtained PAFs have rigid conjugated backbones, high specific surface area, and excellent stability. The prepared PAF‐154 and PAF‐155 have been successfully applied in the perovskite solar cells (PSCs) by doping into the perovskite layer. The champion PSC devices afford a power conversion efficiency...
Fully conjugated porous aromatic frameworks (PAFs) have been constructed through Gilch reaction. The obtained PAFs have rigid conjugated backbones, high specific surface area, and excellent stability. The prepared PAF‐154 and PAF‐155 have been successfully applied in the perovskite solar cells (PSCs) by doping into the perovskite layer. The champion PSC devices afford a power conversion efficiency...