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Two‐dimensional (2D) hybrid perovskite materials have been widely used for polarization‐sensitive photodetection due to their fascinating optical and physical attributes. However, studies on those materials that enable strong polarized‐light activities under a weak‐light condition remain quite scarce. Here, by tailoring aromatic cation into 3D prototype, we have successfully obtained a new 2D hybrid...
Layered heterostructures of different 2D building blocks have invigorated the booming of 2D materials toward high‐performance optoelectronic devices. However, contrary to the typical artificial multi‐component form, the engineering of non‐artificial layered heterostructure into single‐phase crystals and resultant properties are largely overlooked. Here, for the first time, an inch‐sized single crystal...
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