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Rotation around the conjugated C–N bond was investigated through dynamic NMR experiments, employing both 1 H and 13 C spectra, and theoretical calculations (HF and B3LYP with the 6-311+G** and 6-31G** basis sets). Theoretical results predicted slightly distinct gas-phase rotational barriers for the isomers, although inclusion of solvation effects causes the barriers to be essentially...
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