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Ruthenium(II) complexes [(η6‐cymene)RuCl(apypm)]BPh4 with bidentate 2‐amino‐4‐(2‐pyridinyl)pyrimidine (apypm) ligands catalyze the transfer hydrogenation of acetophenone. Their activities are strongly dependent on the substituent pattern of the pyrimidine ring. Complexes bearing a primary amino group in the 2‐position of the pyrimidine ring do not perform the catalysis in terms of a “bifunctional...
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