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For the first time the computed mechanisms for the novel reaction of 2‐naphthol with N‐methyl‐N‐phenylhydrazine, leading to 1‐amino‐2‐naphthol (Tang et al., J Am Chem Soc 2008, 130, 5840), have been investigated using the density functional theory. Four distinct possible pathways were evaluated: two amination mechanisms with the attack of NH2 group respectively at the α‐position C1 and β‐position...
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