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Cation substitution is a promising approach to improve the efficiency of kesterite solar cells. Here, silver has been introduced into Cu2ZnSn(S,Se)4 (CZTSSe) thin film to replace Cu partially and form (Ag xCu1−x)2ZnSn(S,Se)4 (ACZTSSe) through a cost-effective dimethyl sulfoxide-based solution method. Fundamental properties of the mixed Ag–Cu kesterite compound as a function of the Ag/(Ag + Cu) ratio...
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