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The energy density of Ni‐rich cathodes is expected to be further unlocked by increasing the cut‐off voltage to above 4.3 V, which nevertheless come with significantly increased irreversible phase transition and abundant side reactions. In this study, the perovskite oxides enhanced radial‐aligned LiNi0.8Co0.1Mn0.1O2 (NCM811) cathodes are reported, in which the coherent‐growth La2[LiTM]O4 clusters are...
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