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Spin‐dependent charge transport, along with the potential electronic applications, is investigated in chiral 2D iodide hybrid organic/inorganic perovskites (HOIPs) via the chirality‐induced spin selectivity (CISS) effect, paving a new way in spintronics. Despite the high spin‐polarized current enhancement, the intrinsic oxidation tendency of iodide ions brings about severe problems in the stability...
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