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Fine‐tuning of the energy‐level alignment of molecular tunnel junctions is important to maximize their performance. In article number 1706322, Christian A. Nijhuis and co‐workers report junctions based on self‐assembled monolayers that couple to graphene via π–π interactions, which are strong enough to induce electronic function yet with minimal broadening of the molecular orbitals. These junctions...
In molecular electronics, it is important to control the strength of the molecule–electrode interaction to balance the trade‐off between electronic coupling strength and broadening of the molecular frontier orbitals: too strong coupling results in severe broadening of the molecular orbitals while the molecular orbitals cannot follow the changes in the Fermi levels under applied bias when the coupling...
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