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The Li‐plating behavior of Li‐ion batteries under fast‐charging conditions is elusive due to a lack of reliable indicators of the Li‐plating onset. In this work, the relaxation time constant of the charge‐transfer process (τCT) is proposed to be promising for the determination of Li‐plating onset. A novel pulse/relaxation test method enables rapid access to the τCT of the graphite anode during battery...
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