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The stable core–shell Fe@SiO 2 catalysts reported in this paper are highly efficient for the generation of CO x -free H 2 through ammonia decomposition. By tuning the porosity of SiO 2 shells (using C 18 TMS agent) and with the introduction of an appropriate amount of Cs dopant (via pre-deposition as well as post-impregnation), the diffusion efficiency of the...
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