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The anomalous photovoltaic (APV) effect has witnessed great progress from classical ferroelectric photovoltaics to flexo‐photovoltaics. Both call for an extension of the spectral response range. Here, we present a comprehensive study on the ferroelectric, photoelectric, and photovoltaic properties of pure (Bi0.5Na0.5)TiO3 (BNT) and 0.3(Bi0.5Na0.5)TiO3–0.7BiFeO3 (0.3BNT‐0.7BFO) ceramics. The data show...
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