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Boosting the hydrogen evolution reaction (HER) activity of α‐MoB2 at large current densities and in pH‐universal medium is significant for efficient hydrogen production. In this work, Co2B/MoB2 heterostructured nanoclusters are prepared by molten‐salt electrolysis (MSE) and then used as a HER catalyst. The composition, structure, and morphology of Co2B/MoB2 can be modulated by altering the stoichiometries...