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Soft, stretchable, tough, and adhesive elastomers are developed based on the metal‐ionic crosslinked double network structure, where the metal ion coordination of sulfonated poly(phenylene oxide) (SPPO) is used for the first network and the soft chemical crosslinked poly(ethyl acrylate) (PEA) is used for the second network. The influence of SPPO content on the tensile, cyclic tensile, adhesive, and...
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