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The sharp loss‐in‐capacity in CO2 capture as a result of sintering is a major drawback for CaO‐based sorbents used in the calcium looping process. The decoration of inert supports effectively stabilizes the cyclic CO2 capture performance of CaO‐based sorbents via sintering mitigation. A range of Al‐decorated and Al/Mg co‐decorated CaO‐based sorbents were synthesized via an easily scaled‐up spray‐drying...
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