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Natural light‐harvesting (LH) systems can divide identical dyes into unequal aggregate states, thereby achieving intelligent “allocation of labor”. From a synthetic point of view, the construction of such kinds of unequal and integrated systems without the help of proteinaceous scaffolding is challenging. Here, we show that four octatetrayne‐bridged ortho‐perylene diimide (PDI) dyads (POPs) self‐assemble...
Natural light‐harvesting (LH) systems can divide identical dyes into unequal aggregate states, thereby achieving intelligent “allocation of labor”. From a synthetic point of view, the construction of such kinds of unequal and integrated systems without the help of proteinaceous scaffolding is challenging. Here, we show that four octatetrayne‐bridged ortho‐perylene diimide (PDI) dyads (POPs) self‐assemble...