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Focusing on the bottleneck of molecularly engineered organic semiconductors, a breakthrough is made to tune the electronic properties of organic semiconductors from p‐type to n‐type by using fluorinated metal phthalocyanines as examples. The experimentally observed p‐type to n‐type transition characteristics of single‐crystal field‐effect devices result from a combination of extrinsic and intrinsic...
In article number 1605053, Hui Jiang, Wenping Hu, Christian Kloc, and co‐workers demonstrate that by adjusting the substitutional symmetry of fluorinated metal phthalocyanines, the charge‐carrier type can be tuned from p‐type to n‐type. Only hole transport can be observed in metal phthalocyanine (CuPc) while only electron transport can be found in fully fluorinated metal phthalocyanines (F16CuPc)...
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