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The second harmonic generation ability of new chiral thiolate salts is investigated. Aromatic thiolate anions ArS − are expected from semi-empirical calculations with PM3 parameterization of the MNDO Hamiltonian to possess higher intrinsic polarizabilities than the parent neutral thiols ArSH.Salts associating (hyper)polarizable aromatic thiolate anions with chiral cations, which ensure the...
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