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Magnetoelectric coupling is achieved near room temperature in a spin crossover FeII molecule‐based compound, [Fe(1bpp)2](BF4)2. Large atomic displacements resulting from Jahn–Teller distortions induce a change in the molecule dipole moment when switching between high‐spin and low‐spin states leading to a step‐wise change in the electric polarization and dielectric constant. For temperatures in the...
Magnetoelectric coupling is achieved near room temperature in a spin crossover FeII molecule‐based compound, [Fe(1bpp)2](BF4)2. Large atomic displacements resulting from Jahn–Teller distortions induce a change in the molecule dipole moment when switching between high‐spin and low‐spin states leading to a step‐wise change in the electric polarization and dielectric constant. For temperatures in the...