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The rotational spectrum of acrylonitrile was studied up to 1.67THz by recording and analysing several extended spectral segments spanning a total of over 540GHz. The spectra were obtained with cascaded harmonic multiplication techniques, and the ground state data set was extended to over 3000 lines, J=129, and includes transitions up to Ka=30. At high-J and K a several manifestations of a...
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