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The hydrogenation of CO2 was investigated on Ga2O3-promoted Pd/SiO2 catalyts and mechanical mixtures of Ga2O3/SiO2 and Pd/SiO2 catalysts (H2/CO2 = 3; P = 3.0 MPa; T = 523 K). By means of the latter it was possible to demonstrate that atomic hydrogen, Hs, can be generated by Pd0 far from Ga2O3, and move (spill-over) there to reach the other reactive species (formates) and complete the reaction cycle...
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