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Layers depleted of Li‐ions in solid‐state electrolytes have a substantial impact on the performance of all‐solid‐state batteries. In article number 2100585, Aliaksandr S. Bandarenka and co‐workers develop a practical strategy to measure the thickness of such space charge layers and the corresponding concentration of Li‐ions by applying spectroscopic ellipsometry to emerging battery materials.
The future of mobility depends on the development of next‐generation battery technologies, such as all‐solid‐state batteries. As the ionic conductivity of solid Li+‐conductors can, in some cases, approach that of liquid electrolytes, a significant remaining barrier faced by solid‐state electrolytes (SSEs) is the interface formed at the anode and cathode materials, with chemical instability and physical...
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